Libra heart perfect zodiac signs are gemini, water bearer, and aries. When it comes to matters of the heart, Libra seeks equilibrium and compatibility above all else. Gemini can provide stimulation and fun to the connection, while Aquarius shares Libra's appreciation for wisdom and innovation. The Ram, known for their intensity, can ignite a spark in Libra's spirit. Libra and these signs create a balanced and fulfilling union.